You need to create start shortcut icons on the desktop for each profile! Go to the Iron install directory, Right click the iron.exe file, and then tell it to "Send to -- Desktop(create shortcut)'. Or Right Click>New>Shortcut, and fill in the blanks(I find it is easier to create the shortcut from the Install folder).
Now you need to modify the Target box to point to a Profile.
Here is an example
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"C:\Program Files\SRWare Iron\iron.exe" --user-data-dir="C:\Documents and Settings\<<<USER-NAME>>>\Local Settings\Application Data\Chromium\User Data\Iron14"
This is the portion that tells where the Profile is located.
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--user-data-dir="C:\Documents and Settings\<<<USER-NAME>>>\Local Settings\Application Data\Chromium\User Data\Iron14"
Once you get one working, COPY it and PASTE to the Desktop, and modify that last portion to the second profile. I have about 5 I use.
This is the way I learned to do it. Other users may have a better way.